Behavior of selected hydrolyzed and dehydrated products during hydrothermal carbonization of biomass.
Identifieur interne : 002352 ( Main/Exploration ); précédent : 002351; suivant : 002353Behavior of selected hydrolyzed and dehydrated products during hydrothermal carbonization of biomass.
Auteurs : M Toufiq Reza [Allemagne] ; Benjamin Wirth [Allemagne] ; Ulf Lüder [Allemagne] ; Maja Werner [Allemagne]Source :
- Bioresource technology [ 1873-2976 ] ; 2014.
Descripteurs français
- KwdFr :
- Biomasse (MeSH), Biotechnologie (méthodes), Carbone (analyse), Carbone (pharmacologie), Cellulose (composition chimique), Charbon de bois (composition chimique), Cinétique (MeSH), Déchets (analyse), Eau (pharmacologie), Furfural (analyse), Hydrolyse (MeSH), Oxygène (analyse), Populus (composition chimique), Populus (effets des médicaments et des substances chimiques), Spectroscopie infrarouge à transformée de Fourier (MeSH), Température (MeSH), Triticum (composition chimique), Triticum (effets des médicaments et des substances chimiques).
- MESH :
- analyse : Carbone, Déchets, Furfural, Oxygène.
- composition chimique : Cellulose, Charbon de bois, Populus, Triticum.
- effets des médicaments et des substances chimiques : Populus, Triticum.
- méthodes : Biotechnologie.
- pharmacologie : Carbone, Eau.
- Biomasse, Cinétique, Hydrolyse, Spectroscopie infrarouge à transformée de Fourier, Température.
English descriptors
- KwdEn :
- Biomass (MeSH), Biotechnology (methods), Carbon (analysis), Carbon (pharmacology), Cellulose (chemistry), Charcoal (chemistry), Furaldehyde (analysis), Hydrolysis (MeSH), Kinetics (MeSH), Oxygen (analysis), Populus (chemistry), Populus (drug effects), Spectroscopy, Fourier Transform Infrared (MeSH), Temperature (MeSH), Triticum (chemistry), Triticum (drug effects), Waste Products (analysis), Water (pharmacology).
- MESH :
- chemical , analysis : Carbon, Furaldehyde, Oxygen, Waste Products.
- chemical , chemistry : Cellulose, Charcoal.
- chemistry : Populus, Triticum.
- drug effects : Populus, Triticum.
- methods : Biotechnology.
- chemical , pharmacology : Carbon, Water.
- Biomass, Hydrolysis, Kinetics, Spectroscopy, Fourier Transform Infrared, Temperature.
Abstract
In this study, effects of reaction temperature and reaction time on both solid hydrochar and HTC process liquid products were studied for hydrothermal carbonization (HTC) of cellulose, wheat straw, and poplar. A novel slurry sampling system was designed and used with an 18.6L Parr reactor for 0-480 min in 200, 230, and 260 °C. Sugars (sucrose, glucose, and fructose), HMF, and furfural were found maximum in lower HTC temperature and time. However, they degrade following first order degradation kinetics. Activation energies of total sugars (glucose, fructose, sucrose, and xylose), furfural, and HMF for straw and poplar were 95-127, 130-135, and 74-90 kJ mol(-1), respectively and individuals were lower for HTC of cellulose than others. Organic acids (acetic acid, formic acid, and lactic acid) and phenolic compounds (phenol, catechol, and guaiacol) were increasing with higher HTC severity.
DOI: 10.1016/j.biortech.2014.07.010
PubMed: 25063978
Affiliations:
Links toward previous steps (curation, corpus...)
Le document en format XML
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Electronic address: treza@atb-potsdam.de.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>APECS Group, Leibniz Institute for Agricultural Engineering (ATB), Max-Eyth-Allee 100, Potsdam 14469</wicri:regionArea><placeName><region type="land" nuts="2">Brandebourg</region><settlement type="city">Potsdam</settlement></placeName></affiliation></author><author><name sortKey="Wirth, Benjamin" sort="Wirth, Benjamin" uniqKey="Wirth B" first="Benjamin" last="Wirth">Benjamin Wirth</name><affiliation wicri:level="3"><nlm:affiliation>APECS Group, Leibniz Institute for Agricultural Engineering (ATB), Max-Eyth-Allee 100, Potsdam 14469, Germany.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>APECS Group, Leibniz Institute for Agricultural Engineering (ATB), Max-Eyth-Allee 100, Potsdam 14469</wicri:regionArea><placeName><region type="land" nuts="2">Brandebourg</region><settlement type="city">Potsdam</settlement></placeName></affiliation></author><author><name sortKey="Luder, Ulf" sort="Luder, Ulf" uniqKey="Luder U" first="Ulf" last="Lüder">Ulf Lüder</name><affiliation wicri:level="3"><nlm:affiliation>APECS Group, Leibniz Institute for Agricultural Engineering (ATB), Max-Eyth-Allee 100, Potsdam 14469, Germany.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>APECS Group, Leibniz Institute for Agricultural Engineering (ATB), Max-Eyth-Allee 100, Potsdam 14469</wicri:regionArea><placeName><region type="land" nuts="2">Brandebourg</region><settlement type="city">Potsdam</settlement></placeName></affiliation></author><author><name sortKey="Werner, Maja" sort="Werner, Maja" uniqKey="Werner M" first="Maja" last="Werner">Maja Werner</name><affiliation wicri:level="3"><nlm:affiliation>APECS Group, Leibniz Institute for Agricultural Engineering (ATB), Max-Eyth-Allee 100, Potsdam 14469, Germany.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>APECS Group, Leibniz Institute for Agricultural Engineering (ATB), Max-Eyth-Allee 100, Potsdam 14469</wicri:regionArea><placeName><region type="land" nuts="2">Brandebourg</region><settlement type="city">Potsdam</settlement></placeName></affiliation></author></analytic><series><title level="j">Bioresource technology</title><idno type="eISSN">1873-2976</idno><imprint><date when="2014" type="published">2014</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Biomass (MeSH)</term><term>Biotechnology (methods)</term><term>Carbon (analysis)</term><term>Carbon (pharmacology)</term><term>Cellulose (chemistry)</term><term>Charcoal (chemistry)</term><term>Furaldehyde (analysis)</term><term>Hydrolysis (MeSH)</term><term>Kinetics (MeSH)</term><term>Oxygen (analysis)</term><term>Populus (chemistry)</term><term>Populus (drug effects)</term><term>Spectroscopy, Fourier Transform Infrared (MeSH)</term><term>Temperature (MeSH)</term><term>Triticum (chemistry)</term><term>Triticum (drug effects)</term><term>Waste Products (analysis)</term><term>Water (pharmacology)</term></keywords><keywords scheme="KwdFr" xml:lang="fr"><term>Biomasse (MeSH)</term><term>Biotechnologie (méthodes)</term><term>Carbone (analyse)</term><term>Carbone (pharmacologie)</term><term>Cellulose (composition chimique)</term><term>Charbon de bois (composition chimique)</term><term>Cinétique (MeSH)</term><term>Déchets (analyse)</term><term>Eau (pharmacologie)</term><term>Furfural (analyse)</term><term>Hydrolyse (MeSH)</term><term>Oxygène (analyse)</term><term>Populus (composition chimique)</term><term>Populus (effets des médicaments et des substances chimiques)</term><term>Spectroscopie infrarouge à transformée de Fourier (MeSH)</term><term>Température (MeSH)</term><term>Triticum (composition chimique)</term><term>Triticum (effets des médicaments et des substances chimiques)</term></keywords><keywords scheme="MESH" type="chemical" qualifier="analysis" xml:lang="en"><term>Carbon</term><term>Furaldehyde</term><term>Oxygen</term><term>Waste Products</term></keywords><keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Cellulose</term><term>Charcoal</term></keywords><keywords scheme="MESH" qualifier="analyse" xml:lang="fr"><term>Carbone</term><term>Déchets</term><term>Furfural</term><term>Oxygène</term></keywords><keywords scheme="MESH" qualifier="chemistry" xml:lang="en"><term>Populus</term><term>Triticum</term></keywords><keywords scheme="MESH" qualifier="composition chimique" xml:lang="fr"><term>Cellulose</term><term>Charbon de bois</term><term>Populus</term><term>Triticum</term></keywords><keywords scheme="MESH" qualifier="drug effects" xml:lang="en"><term>Populus</term><term>Triticum</term></keywords><keywords scheme="MESH" qualifier="effets des médicaments et des substances chimiques" xml:lang="fr"><term>Populus</term><term>Triticum</term></keywords><keywords scheme="MESH" qualifier="methods" xml:lang="en"><term>Biotechnology</term></keywords><keywords scheme="MESH" qualifier="méthodes" xml:lang="fr"><term>Biotechnologie</term></keywords><keywords scheme="MESH" qualifier="pharmacologie" xml:lang="fr"><term>Carbone</term><term>Eau</term></keywords><keywords scheme="MESH" type="chemical" qualifier="pharmacology" xml:lang="en"><term>Carbon</term><term>Water</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Biomass</term><term>Hydrolysis</term><term>Kinetics</term><term>Spectroscopy, Fourier Transform Infrared</term><term>Temperature</term></keywords><keywords scheme="MESH" xml:lang="fr"><term>Biomasse</term><term>Cinétique</term><term>Hydrolyse</term><term>Spectroscopie infrarouge à transformée de Fourier</term><term>Température</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">In this study, effects of reaction temperature and reaction time on both solid hydrochar and HTC process liquid products were studied for hydrothermal carbonization (HTC) of cellulose, wheat straw, and poplar. A novel slurry sampling system was designed and used with an 18.6L Parr reactor for 0-480 min in 200, 230, and 260 °C. Sugars (sucrose, glucose, and fructose), HMF, and furfural were found maximum in lower HTC temperature and time. However, they degrade following first order degradation kinetics. Activation energies of total sugars (glucose, fructose, sucrose, and xylose), furfural, and HMF for straw and poplar were 95-127, 130-135, and 74-90 kJ mol(-1), respectively and individuals were lower for HTC of cellulose than others. Organic acids (acetic acid, formic acid, and lactic acid) and phenolic compounds (phenol, catechol, and guaiacol) were increasing with higher HTC severity.</div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" Owner="NLM"><PMID Version="1">25063978</PMID><DateCompleted><Year>2015</Year><Month>05</Month><Day>14</Day></DateCompleted><DateRevised><Year>2017</Year><Month>09</Month><Day>26</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1873-2976</ISSN><JournalIssue CitedMedium="Internet"><Volume>169</Volume><PubDate><Year>2014</Year><Month>Oct</Month></PubDate></JournalIssue><Title>Bioresource technology</Title><ISOAbbreviation>Bioresour Technol</ISOAbbreviation></Journal><ArticleTitle>Behavior of selected hydrolyzed and dehydrated products during hydrothermal carbonization of biomass.</ArticleTitle><Pagination><MedlinePgn>352-361</MedlinePgn></Pagination><ELocationID EIdType="pii" ValidYN="Y">S0960-8524(14)00975-4</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.1016/j.biortech.2014.07.010</ELocationID><Abstract><AbstractText>In this study, effects of reaction temperature and reaction time on both solid hydrochar and HTC process liquid products were studied for hydrothermal carbonization (HTC) of cellulose, wheat straw, and poplar. A novel slurry sampling system was designed and used with an 18.6L Parr reactor for 0-480 min in 200, 230, and 260 °C. Sugars (sucrose, glucose, and fructose), HMF, and furfural were found maximum in lower HTC temperature and time. However, they degrade following first order degradation kinetics. Activation energies of total sugars (glucose, fructose, sucrose, and xylose), furfural, and HMF for straw and poplar were 95-127, 130-135, and 74-90 kJ mol(-1), respectively and individuals were lower for HTC of cellulose than others. Organic acids (acetic acid, formic acid, and lactic acid) and phenolic compounds (phenol, catechol, and guaiacol) were increasing with higher HTC severity.</AbstractText><CopyrightInformation>Copyright © 2014 Elsevier Ltd. All rights reserved.</CopyrightInformation></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Reza</LastName><ForeName>M Toufiq</ForeName><Initials>MT</Initials><AffiliationInfo><Affiliation>APECS Group, Leibniz Institute for Agricultural Engineering (ATB), Max-Eyth-Allee 100, Potsdam 14469, Germany. Electronic address: treza@atb-potsdam.de.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Wirth</LastName><ForeName>Benjamin</ForeName><Initials>B</Initials><AffiliationInfo><Affiliation>APECS Group, Leibniz Institute for Agricultural Engineering (ATB), Max-Eyth-Allee 100, Potsdam 14469, Germany.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Lüder</LastName><ForeName>Ulf</ForeName><Initials>U</Initials><AffiliationInfo><Affiliation>APECS Group, Leibniz Institute for Agricultural Engineering (ATB), Max-Eyth-Allee 100, Potsdam 14469, Germany.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Werner</LastName><ForeName>Maja</ForeName><Initials>M</Initials><AffiliationInfo><Affiliation>APECS Group, Leibniz Institute for Agricultural Engineering (ATB), Max-Eyth-Allee 100, Potsdam 14469, Germany.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType><PublicationType UI="D013485">Research Support, Non-U.S. Gov't</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2014</Year><Month>07</Month><Day>08</Day></ArticleDate></Article><MedlineJournalInfo><Country>England</Country><MedlineTA>Bioresour Technol</MedlineTA><NlmUniqueID>9889523</NlmUniqueID><ISSNLinking>0960-8524</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D014866">Waste Products</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="C540010">biochar</NameOfSubstance></Chemical><Chemical><RegistryNumber>059QF0KO0R</RegistryNumber><NameOfSubstance UI="D014867">Water</NameOfSubstance></Chemical><Chemical><RegistryNumber>16291-96-6</RegistryNumber><NameOfSubstance UI="D002606">Charcoal</NameOfSubstance></Chemical><Chemical><RegistryNumber>7440-44-0</RegistryNumber><NameOfSubstance UI="D002244">Carbon</NameOfSubstance></Chemical><Chemical><RegistryNumber>9004-34-6</RegistryNumber><NameOfSubstance UI="D002482">Cellulose</NameOfSubstance></Chemical><Chemical><RegistryNumber>DJ1HGI319P</RegistryNumber><NameOfSubstance UI="D005662">Furaldehyde</NameOfSubstance></Chemical><Chemical><RegistryNumber>S88TT14065</RegistryNumber><NameOfSubstance UI="D010100">Oxygen</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D018533" MajorTopicYN="Y">Biomass</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D001709" MajorTopicYN="N">Biotechnology</DescriptorName><QualifierName UI="Q000379" MajorTopicYN="Y">methods</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D002244" MajorTopicYN="N">Carbon</DescriptorName><QualifierName UI="Q000032" MajorTopicYN="N">analysis</QualifierName><QualifierName UI="Q000494" MajorTopicYN="Y">pharmacology</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D002482" MajorTopicYN="N">Cellulose</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D002606" MajorTopicYN="N">Charcoal</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D005662" MajorTopicYN="N">Furaldehyde</DescriptorName><QualifierName UI="Q000032" MajorTopicYN="N">analysis</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D006868" MajorTopicYN="N">Hydrolysis</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D007700" MajorTopicYN="N">Kinetics</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D010100" MajorTopicYN="N">Oxygen</DescriptorName><QualifierName UI="Q000032" MajorTopicYN="N">analysis</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D032107" MajorTopicYN="N">Populus</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName><QualifierName UI="Q000187" MajorTopicYN="N">drug effects</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D017550" MajorTopicYN="N">Spectroscopy, Fourier Transform Infrared</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D013696" MajorTopicYN="Y">Temperature</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D014908" MajorTopicYN="N">Triticum</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName><QualifierName UI="Q000187" MajorTopicYN="N">drug effects</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D014866" MajorTopicYN="N">Waste Products</DescriptorName><QualifierName UI="Q000032" MajorTopicYN="N">analysis</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D014867" MajorTopicYN="N">Water</DescriptorName><QualifierName UI="Q000494" MajorTopicYN="Y">pharmacology</QualifierName></MeshHeading></MeshHeadingList><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Degradation kinetics</Keyword><Keyword MajorTopicYN="N">HTC process liquid</Keyword><Keyword MajorTopicYN="N">Hydrochar</Keyword><Keyword MajorTopicYN="N">Hydrothermal carbonization</Keyword><Keyword MajorTopicYN="N">Lignocellulosic biomass</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2014</Year><Month>05</Month><Day>28</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2014</Year><Month>06</Month><Day>30</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2014</Year><Month>07</Month><Day>01</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2014</Year><Month>7</Month><Day>27</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2014</Year><Month>7</Month><Day>27</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2015</Year><Month>5</Month><Day>15</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">25063978</ArticleId><ArticleId IdType="pii">S0960-8524(14)00975-4</ArticleId><ArticleId IdType="doi">10.1016/j.biortech.2014.07.010</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list><country><li>Allemagne</li></country><region><li>Brandebourg</li></region><settlement><li>Potsdam</li></settlement></list><tree><country name="Allemagne"><region name="Brandebourg"><name sortKey="Reza, M Toufiq" sort="Reza, M Toufiq" uniqKey="Reza M" first="M Toufiq" last="Reza">M Toufiq Reza</name></region><name sortKey="Luder, Ulf" sort="Luder, Ulf" uniqKey="Luder U" first="Ulf" last="Lüder">Ulf Lüder</name><name sortKey="Werner, Maja" sort="Werner, Maja" uniqKey="Werner M" first="Maja" last="Werner">Maja Werner</name><name sortKey="Wirth, Benjamin" sort="Wirth, Benjamin" 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